100 years of physical chemistry - download pdf or read online

By Royal Society of Chemistry (Great Britain)

ISBN-10: 0854049827

ISBN-13: 9780854049820

ISBN-10: 0854049878

ISBN-13: 9780854049875

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Kuntz, J. Valldorf, Z. Phys. , 1988,S, 195; H-U. Bohmer and S. D. Peyerimhoff, Z. Phys. D, 1989,11,249. 28 R. N. Bhatt and T. M. Rice, Phys. Rev. B, 1979,20,466. 29 L. A. Turkevich and M. H. Cohen, Phys. Rev. , 1964, 53, 232; J . Non-cryst. Solids, 1984,61&62, 13; J . Phys. , 1984, 26 88,3751. 30 N. W. Ashcroft, Science, 1989,340,345. 31 C. Castellani, G. Kotliar and P. A. Lee, Phys. Rev. , 1987, 59,323 and references therein. 32 M. Lakner and H. v. Lohneysen, Phys. Rev. , 1989,63,648. 33 N. F.

This change in chemical binding has a strong influence, not only on the physical properties of mercury clusters, but also on the properties of expanded Hg,’ and on Hg layers on solid2 and liquid3 surfaces. For a rigid cluster the electronic states are discreet and not continuous as in fig. 1. Also the term ‘band’ for a bundle of electronic states will be used repeatedly in this paper, although ‘incipient band’ might be better. As the clusters discussed here are relatively hot, possibly liquid, any discreet structure will be broadened into some form of structured ‘band’.

Although our data agree in general with those of ref. (5) and (6), Rademann' arrives at very different conclusions, as discussed below. The large decrease of the ionisation energies for small n is due to the strongly bound dimer ion H g i . The fragmentation effects due to its strong binding can be expected to be less severe than for the kindred rare-gas case,', as the ratio of neutral to ionic dissociation energies is higher. For very small n we expect to have some fragmentation even close to threshold, although we presently do not have a means of quantifying this expectation.

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100 years of physical chemistry by Royal Society of Chemistry (Great Britain)


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